Application of Anaerobic and Multiple-Electron-Acceptor Bioremediation to Chlorinated Aliphatic Subsurface Contamination

Principal Investigator

G.F. Parkin, University of Iowa

Goal

The goal of this project is to advance understanding of anaerobic and mixed-electron acceptor bioremediation of chlorinated aliphatics to a level that full-scale evaluation of these processes is possible. If successful, field-scale evaluation of technologies developed in this research will be pursued.

Rationale

The U.S. EPA Hazardous Substance Research Centers and national agencies such as the Department of Defense and Department of Energy have identified research on remediation processes for chlorinated aliphatic-contaminated subsurfaces as a high priority. A promising technique is use of in situ bioremediation, and full-scale evaluations of this process are ongoing at trichloroethene-contaminated sites. All of these efforts have focused on use of aerobic bacteria, particularly methanotrophs. However, several of the chlorinated aliphatics of greatest concern are not degraded by aerobic bacteria. Unlike aerobic biological processes, anaerobic biotransformations of all chlorinated aliphatics occur. This lack of specificity, coupled with the fact that most contaminated aquifers are anaerobic, may make anaerobic bioremediation an alternative or supplement to aerobic processes.

Approach

This research will focus on three chlorinated aliphatics that are not degraded by aerobic bacteria: perchloroethene, 1,1,1-trichloroethane, and carbon tetrachloride. If successful, field-scale evaluation of technologies developed in this research will be pursued. In order to accurately assess potential for anaerobic or combined electron acceptor bioremediation technology, all experimental systems will be operated under conditions similar to those observed in contaminated aquifers. Additionally, soil cores will be obtained from contaminated sites as a source of organisms that are indigenous to contaminated areas. These cultures may be considerably different than those obtained from anaerobic digesters and may contain organisms particularly suited for chlorinated aliphatic degradation.

Status

All the necessary equipment has been updated and all experimental systems are functioning properly. Preliminary kinetic experiments have been completed and detailed experiments are continuing. Preliminary studies using only anaerobic biofilm columns have essentially been completed. Aerobic columns have been attached to anaerobic columns and chlorinated compounds have been fed to these systems for more than six months. A change in the anticipated funding has made it uncertain if the investigators will be able to complete studies on identification of organisms that are able to convert chlorinated aliphatics to nonobjectionable products or on the effects of nonaqueous phase chlorinated aliphatics on the extent of degradation and toxicity. This project is in its third year.

Clients/Users

Results from this research will be of interest to other researchers, U.S. Environmental Protection Agency, U.S. Department of Defense, U.S. Department of Energy, and others.

Keywords

Anaerobic, bioremediation, chlorinated aliphatics, mixed-electron acceptor.


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